何乐

教授、博士生导师

何乐，教授博士生导师2008年于南京大学获得学士学位，苏州大学功能纳米与软物质研究院，被聘为教授、博士生导师。

人物经历

2008年于南京大学获得学士学位，2013年于美国加州大学河滨分校获得化学博士学位。2013年至2015年在加拿大多伦多大学从事博士后研究。2015年9月加入苏州大学功能纳米与软物质研究院，被聘为教授、博士生导师。入选国家级青年人才计划、江苏省“双创计划”、江苏省“333人才工程”第二层次、江苏省优青、江苏省六大人才高峰高层次人才。2023年11月起担任苏州大学科学技术研究院院长。

研究领域

本课题组的研究集中于气相光催化二氧化碳还原，致力于解决现有体系在活性、选择性与稳定性方面存在的不足，加深对光催化机制与反应机理的理解。

主要成果和贡献

获奖荣誉

代表论文

Song, R.†; Zhao, G.†; Restrepo-Florez, J. M.; Viasus, C. J.; Chen, Z.; Ai, C.; Wang, A.; Jing, D.; Tountas, A. A.; Mao, C.; Li, C.; Shen, J.; Cai, G.; Qiu, C.; Ye, J.; Fu, Y.; Wang, L.; Sun, J.; Xu, Y.-F.; Li, Z.; Nguyen, N. T.; Maravelias, C.; He, L.*; Zhang, X.*; Ozin, G. A.*, Solar Ethene: Selective Photocatalytic Dehydrogenation of Ethane, Nat. Energy, 2024, In Press. (†equal contribution)

Xiao, Y.; Feng, K.; Dawson, G.; Tolstoy, V. P.; An, X.*; Li, C.*; He, L.*, A feasible interlayer strategy for simultaneous light and heat management in photothermal catalysis, iScience, 2024, In Press.

Hu, X.†; Zhu, Z.†; Zhou, Y.†; Liu, S.; Wu, C.; Wang, J.; Shen, Y.; Yan, T.; Zhang, L.; Chen, J.; Feng, K.; Genest, A.; Rupprechter, G.; An, X.*; Li, C.*; He, L.*, Enhanced photochemical eﬀects of plasmonic cluster catalysts through aggregated nanostructures, Green Chem., 2024, In Press. (†equal contribution)

Wang, J.†; Zhu, Z.†; Feng, K.†; Liu, S.; Zhou, Y.; Urooj, I.; He, J.; Wu, Z.; Shen, J.; Hu, X.; Chen, Z.; Dong, X.; Sohail, M.; Ma, Y.; Chen, J.; Li, C.*; An, X.*; He, L.*, Anisotropic Plasmon Resonance Enables Spatially Controlled Photothermal and Photochemical Effects in Hot Carrier-Driven Catalysis, Chin. J. Chem., 2024, In Press. (†equal contribution)

Zhang, L.†; An, X.†; Feng, K.†; Li, J.; Liu, J.; Chen, J.; Li, C.*; Zhang, X.*; He, L.*, Non-Photochemical Origin of Selectivity Difference between Light and Dark Catalytic Conditions, ACS Appl. Mater. Interfaces, 2024, 16, 21987–21996. (†equal contribution)

Zhong, B.†; Cai, M.†; Liu, S.; He, J.; Wang, J.; Feng, K.; Tolstoy, V. P.; Jiang, L.; Li, C.*; An, X.*; He L.*, Modulation of the Structure-function Relationship of the “nano-greenhouse effect” towards Optimized Supra-photothermal Catalysis, Chem. Asian J., 2024, 19, e202301077. (†equal contribution)

Zhang, C.†; Wu, Z.†; Shen, J.; He, L.*; Sun, W.*, Silicon Nanostructure Arrays: An Emerging Platform for Photothermal CO2 Catalysis, Acta Phys. -Chim. Sin., 2024, 40, 2304004. (†equal contribution)

Cai, M.†; Li, C.†; An, X.†; Zhong, B.; Zhou, Y.; Feng, K.; Wang, S.; Zhang, C.; Xiao, M.; Wu, Z.; He, J.; Wu, C.; Shen, J.; Zhu, Z.; Feng, K.; Zhong, J.; He, L.*, Supra-photothermal CO2 methanation over greenhouse-like plasmonic superstructures of ultra-small cobalt nanoparticles, Adv. Mater., 2024, 36, 2308859. (†equal contribution)

Zhu, Z.†; Tang, R.†; Li, C.*; An, X.*; He, L.*, Promises of Plasmonic Antenna-Reactor Systems in Gas-Phase CO2 Photocatalysis, Adv. Sci., 2023, 10, 2302568. (†equal contribution)

Xi, Y.†; Cai, M.†; Wu, Z.; Zhu, Z.; Shen, J.; Zhang C.; Tang, R.; An, X.*; Li, C.*; He, L.*, Identiﬁcation of photochemical effects in Ni-based photothermal catalysts, Chin. J. Struct. Chem., 2023, 42, 100071. (†equal contribution)

Wu, Z.†; Shen, J.†; Li, C.; Zhang, C.; Wu, C.; Li, Z.; An, X.*; He, L.*, Niche Applications of MXene Materials in Photothermal Catalysis, Chemistry, 2023, 5, 492-510. (†equal contribution)

Wu, Z.†; Shen, J.†; Li, C.*; Zhang, C.; Feng, K.; Wang, Z.; Wang, X.; Meira, D.; Cai, M.; Zhang, D.; Wang, S.; Chu, M.; Chen, J.; Xi, Y.; Zhang, L.; Sham, T.; Genest, A.; Rupprechter, G.; Zhang, X.*; He, L.*, Stabilization of Exposed Metal Nanocrystals in High-Temperature Heterogeneous Catalysis, ACS Nano, 2023, 17, 1550-1559. (†equal contribution)

Zhong, G.; Zhao, R.; Shi, Y.; Li, C.; He, L.*; He, L.; Huang, Y.*; Thermal Shock Synthesis of Carbon Nanotubes Supporting Small-sized Rhenium Nanoparticles for Efficient Electrocatalytic Hydrogen Evolution, Rare Met., 2023, 42, 2166-2173.

Zhu, Z.†; Feng, K.†; Li, C.*; Tang, R.; Xiao, M.; Song, R.; Yang, D.; Yan, B.*; He, L.*, Stabilization of Exposed Metal Nanocrystals in High-Temperature Heterogeneous Catalysis, Adv. Mater. 2022, 34, 2108727. (†equal contribution)

Wang, S.†; Zhang, D.†; Wang, W.; Zhong, J.; Feng, K.; Wu, Z.; Du, B.; He, J.; Li, Z.; He, L.*; Sun, W.*; Yang, D.*; Ozin, G.*, Grave-to-cradle Upcycling of Ni from Electroplating Wastewater to Photothermal CO2 Catalysis, Nat. Commun., 2022, 13, 5305.

Zhang, C.†; Kang, Q.†; Chu, M.; He, L.*; Chen, J.*, Solar-Driven Catalytic Plastic Upcycling, Trends Chem., 2022, 4, 822-834.

Shen, X.; Li, C.*; Wu, Z.; Tang, R.; Shen, J.; Chu, M.; Xu, A.; Zhang, B.*; He, L.*; Zhang, X., Rationally Designed Nanoarray Catalysts for Boosted Photothermal CO2 Hydrogenation, Nanoscale, 2022, 14, 11568-11574.

Chen, Z.†; Li, H.†; Li, C.*; Liu, J.; Hua, W.; Zhang, X.; Zhang, C.; Xiao, M.; Xu, A.B.; He, L.*; Zhang, X.*, Shear-induced alignment of low-aspect-ratio nanorods for modulations of multiple optical properties, J. Mater. Chem. C, 2022, 10, 9478-9483

Guo, J.†*; Song, R.†; Li, Z.; Pan, D.; Xie, H.; Ba, Y.; Xie, M.; Fan, S.; Yang, X.; Zhang, H.; Yu, H.; Zhang, S.; Du, J.*; He, L.*; Wang, L.*, Gold Decorated Hydroxyapatite–CeO2 Enabled Surface Frustrated Lewis Pairs for CO Oxidation, Adv. Energy Sustainability Res., 2022, 3, 2200106.

Zhu, Z.†; Hu, X.†; An, X.; Xiao, M.; Zhang, L.; Li, C.*; He, L.*, Photothermal catalytic CO2 hydrogenation with high activity and tailored selectivity over monodispersed Pd-Ni nanoalloys, Chem. Asian J., 2022, 17, e202200993.

Shen, J.†; Tang, R.†; Wu, Z.; Wang X.; Chu, M.; Cai, M.; Zhang, C.; Zhang, L.; Yin, K.; He, L.*; Li, C.*, Integrated Photothermal Nanoreactors for Efficient Hydrogenation of CO2, Trans. Tianjin Univ. 2022, 28, 236–244.

Wang, X.; Zhu, Z.; Wu, Z.; Zhang, C.; Chen, Z.; Xiao, M.; Li, C.*; He, L.*, Preparation and Photothermal Catalytic Application of Powder-form Cobalt Plasmonic Superstructures. J. Inorg. Mater., 2022, 37, 22-28.

Cai, M.†; Wu, Z.†; Li, Z.†; Wang, L.; Sun, W.; Tountas, A. A.; Li, C.; Wang, S.; Feng, K.; Xu, A. B.; Tang, S.; Tavasoli, A.; Peng, M.; Liu, W.; Helmy, A. S.; He, L.*; Ozin, G.*; Zhang, X.*, Greenhouse Inspired Supra-Photothermal CO2 Catalysis, Nat. Energy 2021, 6, 807-814. (†equal contribution)

Wu, Z.; Li, C.*; Li, Z.; Feng, K.; Cai, M.; Zhang, D.; Wang, S.; Chu, M.; Zhang, C.; Shen, J.; Huang, Z.; Xiao, Y.; Ozin, G.*; Zhang, X.*; He, L.*, Niobium and Titanium Carbides (MXenes) as Superior Photothermal Supports for CO2 Photocatalysis, ACS Nano 2021, 15, 5696-5705.

Feng, K.; Tian, J.; Guo, M.; Wang, Y.; Wang, S.; Wu, Z.; Zhang, J.; He, L.*; Yan, B.*, Experimentally unveiling the origin of tunable selectivity for CO2 hydrogenation over Ni-based catalysts, Appl. Catal., B 2021, 292, 120191.

Lou, D.†; Zhu, Z.†; Xu, Y. F.†; Li, C.*; Feng, K.; Zhang, D.; Lv, K.; Wu, Z.; Zhang, C.; Ozin, G.*; He, L.*; Zhang, X., A Core-Shell Catalyst Design Boosts the Performance of Photothermal Reverse Water Gas Shift Catalysis, Sci. China Mater. 2021, 64, 2212-2220. (†equal contribution)

Tang, R.†; Zhu, Z.†; Li, C.*; Xiao, M.; Wu, Z.; Zhang, D.; Zhang, C.; Xiao, Y.; Chu, M.; Genest, A.; Rupprechter, G.; Zhang, L.; Zhang, X.*; He, L.*, Ru-Catalyzed Reverse Water Gas Shift Reaction with Near-Unity Selectivity and Superior Stability, ACS Materials Lett. 2021, in press. (†equal contribution)

Xiao, M.; Liu, J.*; Chen, Z.; Liu, W.; Zhang, C.; Yu, Y.; Li, C.*; He, L.*, Magnetic assembly and manipulation of Janus photonic crystal supraparticles from a colloidal mixture of spheres and ellipsoids, J. Mater. Chem. C 2021, 9, 11788-11793.

Lou, D.†; Xu, A.†; Fang, Y.; Cai, M.; Lv, K.; Zhang, D.; Wang, X.; Huang, Y.*; Li, C.*; He, L.*, Cobalt-Sputtered Anodic Aluminum Oxide Membrane for Efficient Photothermal CO2 hydrogenation, ChemNanoMat 2021, 7, 1008-1012.

Shen, J.†; Wu, Z.†; Li, C.*; Zhang, C.; Genest, A.; Rupprechter, G.; He, L.*, Emerging applications of MXene materials in CO2 photocatalysis, Flatchem 2021, 28, 100252. (†equal contribution)

Wu, Z.; Zhang, C.; Li, C.*; He, L.*, Research Progress on Magnetically Responsive Smart Optical Nanomaterials, Materials China 2021, 40, 1-10.

Zhang, D.†; Lv, K.†; Li, C.; Fang, Y.; Wang, S.; Chen, Z.; Wu, Z.; Guan, W.; Lou, D.; Sun, W.*; Yang, D.; He, L.*; Zhang, X.*, All-Earth-Abundant Photothermal Silicon Platform for CO2 Catalysis with Nearly 100% Sunlight Harvesting Ability, Solar RRL 2021, 5, 2000387. (†equal contribution)

Feng, K.†; Wang, S.†; Zhang, D.†; Wang, L.; Yu, Y.; Feng, K.; Li, Z.; Zhu, Z.; Li, C.; Cai, M.; Wu, Z.; Kong, N.; Yan, B.; Zhong, J.*; Zhang, X.*; Ozin, G.*; He, L.*, Cobalt Plasmonic Superstructures Enable Almost 100% Broadband Photon Efficient CO2 Photocatalysis, Adv. Mater. 2020, 32, 2000014. (†equal contribution)

Fang, Y.†; Lv, K.†; Li, Z.; Kong, N.; Wang, S.; Xu, A.B.; Wu, Z.; Jiang, F.; Li, C.*; Ozin, G.*; He, L.*, Solution-Liquid-Solid Growth and Catalytic Applications of Silica Nanorod Arrays, Adv. Sci. 2020, 7, 2000310. (†equal contribution)

Li, C.†; Zhang, J.†; Wang, S.; Zhu, Z.; Li, H.*; Xu, A. B.; Yu, Y.; Wang, X.; Yao, J.; Wang, L.*; Solovev, A. A.; He, L.*, Silica Nanocapsules with Unusual Shapes Accessed by Simultaneous Growth of the Template and Silica Nanostructure, Chem. Mater. 2020, 32, 575-581. (†equal contribution)

Cai, M; Li, C.*; He, L.*, Enhancing Photothermal CO2 Catalysis by Thermal Insulating Substrates, Rare Met. 2020, 39, 881–886.

Kong, N.; Han, B.; Li, Z.; Fang, Y.; Feng, K.; Wu, Z.; Wang, S.; Xu, A. B.; Yu, Y.; Li, C.*; Lin, Z.*; He, L.*, Ruthenium Nanoparticles Supported on Mg(OH)2 Microflowers as Catalysts for Photothermal Carbon Dioxide Hydrogenation, ACS Appl. Nano Mater. 2020, 3, 3028-3033.

Li, C.†; Yu, Y.†; Wang, L.*; Zhang, S.; Liu, J.; Zhang, J.; Xu, A.B.; Wu, Z.; Tong, J.; Wang, S; Xiao, M.; Fang, Y.; Yao, J.; Solovev, A. A.; Dong, B.; He, L.*, A step-by-step strategy for controlled preparations of complex heterostructured colloids, Chem. Mater. 2019, 31, 9513-9521. (†equal contribution)

Liu, J.†; Xiao, M.†; Li, C.*; Li, H.; Wu, Z.; Zhu, Q.; Tang, R.; Xu, A.B.; He, L.*, Rugby-ball-like photonic crystal supraparticles with non-close-packed structures and multiple magneto-optical responses, J. Mater. Chem. C 2019, 7, 15042-15048. (†equal contribution)

Zhang, B.; Jie, J.*; Shao. Z.; Huang, S.; He, L.*; Zhang, X.*, One-step growth of large-area silicon nanowire fabrics for high performance multifunctional wearable sensors, Nano Res. 2019, 12, 2723-2728.

Li, H.†; Li, C.†; Sun, W.; Wang, Y.; Hua, W.; Liu, J.; Zhang, S.; Chen, Z.; Wang, S.; Wu, Z.; Zhu, Q.; Tang, R.; Yu, J.; He, L.*; Ozin, A. G.*; Zhang, X.*, Single-Stimulus-Induced Modulation of Multiple Optical Properties, Adv. Mater. 2019, 31, 1900388. (†equal contribution)

Li, C.†; Yao, J.†; Huang, Y.; Xu, C.; Lou, D.; Wu, Z.; Sun, W.; Zhang, S.; Li, Y.; He, L.*; Zhang, X.*, Salt-Templated Growth of Monodisperse Hollow Nanostructures, J. Mater. Chem. A 2019, 7, 1404-1409. (†equal contribution)

Wang, S.; Li, C.; Chen, Z.; Zhu, Z.; Zhu, Q.; Tang, R.; Sun, W.; He, L.*; Zhang, X.*, Anomalous effect of the aging degree on the ionic permeability of silica shells, RSC Adv. 2018, 8, 38499-38505.

Zhang, S.†; Li, C.†; Zhang, J.; Yu, Y.; Zhou, H.; Tang, R.; Li, Y.; Yu, J.; Du, X.; He, L.*; Zhang, X.*, A general and mild route to highly dispersible anisotropic magnetic colloids for sensing weak magnetic fields, J. Mater. Chem. C 2018, 6, 5528-5535. (†equal contribution)

Wang, L.†; Ghoussoub, M.†; Wang, H.; Dong, Y.; Shao, Y.; Tountas, A.; Wood, T.; Li, H.; Sun, W.; Xia, M.; Li, Y.; Wang, S.; Jia, J.; Qiu, C.; Qian, C.; He, L.*; Zhang, X.*; Ozin, G.*, Photocatalytic Hydrogenation of Carbon Dioxide with High Selectivity to Methanol at Atmospheric Pressure, Joule 2018,2, 1369-1381. (†equal contribution)

Li, C.; Zhang, S.; Zhang, B.; Liu, J.; Zhou, H.; Solovev, A.; Tang, R.; Bao, F.; Yu, J.; Zhang, Q.; Lifshitz, Y.*; He, L.*; Zhang, X.*, Local-Curvature-Controlled Non-Epitaxial Growth of Hierarchical Nanostructures, Angew. Chem. Int. Ed. 2018, 57, 3772-3776.

Wang, L.†; Cai, M.†; Sun, W.*; He, L.*; Zhang, X.*, Promoting Charge Separation in Semiconductor Nanocrystal Superstructures for Enhanced Photocatalytic Activity, Adv. Mater. Interfaces 2018, 5, 1701694. (†equal contribution)

Zhu, Z.†; Zhang, S.†; Li, C.; Zhang, J.; Yu, J.; Du, X.; He, L.*; Zhang, X.*, A Mechanistic Study of Silica-Etching by Hot Water, Phys. Chem. Chem. Phys. 2018, 20, 1440-1446. (†equal contribution)

Cao, M.†; Liu, Q.†; Chen, M.†; Yang, P.; Xu, Y.; Wu, H.; Yu, J.; He, L.*; Zhang, X.*; Zhang, Q.*, Dispersing Hydrophilic Nanoparticles in Nonaqueous Solvents with Superior Long-Term Stability, RSC Adv. 2017, 7, 25535-25541. (†equal contribution)

Yang, P.†; Li, H.†; Zhang, S.; Chen, L.; Zhou, H.; Tang, R.; Zhou, T.; Bao, F.; Zhang, Q.*; He, L.*; Zhang, X.*, Gram-Scale Synthesis of Superparamagnetic Fe3O4 Nanocrystal Clusters with Long-Term Charge Stability for Highly Stable Magnetically Responsive Photonic Crystals, Nanoscale 2016, 8, 19036-19042. (†equal contribution)

Sun, W.†; Qian, C.†; He, L.*; Ghuman, K.; Wong, A.; Jia, J.; O'Brien, P.; Reyes, L.; Wood, T.; Helmy, A.; Mims, C.; Singh, C.; Ozin, G.*, Heterogeneous Reduction of Carbon Dioxide by Hydride-Terminated Silicon Nanocrystals, Nat. Commun. 2016, 7, 12553. (†equal contribution)

He, L.*; Wood, T.; Wu, B.; Dong, Y.; Hoch, L.; Reyes, L.; Wang, D.; Kübel, C.; Qian, C.; Jia, J.; Liao, K.; O'Brien, P.; Sandhel, A.; Loh, J.; Szymanski, P.; Kherani, N.; Sum, T.; Mims, C.; and Ozin, G.*, Spatial Separation of Charge Carriers in In2O3-x(OH)y Nanocrystal Superstructures for Enhanced Gas Phase Photocatalytic Activity, ACS Nano 2016, 10, 5578-5586.

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